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The bistable fluttering response of heavy inverted flags with different aspect ratios ( $AR$ ) is investigated to determine how the vortical structures affect the intermittent vibration response of the flag. A heavy inverted flag in a uniform flow may exhibit several response modes; amongst them are three major modes that occur over an extended velocity range: stationary, large-scale periodic oscillation and one-sided deflected modes. Significant hysteretic bistability is observed at the transition between these modes for all $AR$ , which is notably different from the conventional flag vibration with a fixed leading edge and free trailing edge where no hysteresis is observed at the lower $AR$ limit ( $AR<1$ ). The difference is associated with the distinct roles of vortices around the flag. Experiments with flags made of spring steel are conducted in a wind tunnel, where the flow speed is steadily increased and later decreased to obtain different oscillatory modes of the heavy inverted flags. The experimental results are used to validate the numerical model of the same problem. It is found that different critical velocities exist for increasing and decreasing flow velocities, and there is a sustained hysteresis for all $AR$ controlled by the initiation threshold and growth of the leading-edge and side-edge vortices. The effect of the vortices in the bistable oscillation regime is quantified by formulating a modal force partitioning approach. It is shown that $AR$ can significantly alter the static and dynamic vortex interaction with the flexible plate, thereby changing the flag's hysteresis behaviour and bistable response. 

Low molecular weight hydrogels are made of small molecules that aggregate via noncovalent interactions. Here, comprehensive characterization of the physical and chemical properties of hydrogels made from thioglycolipids of the disaccharides lactose and cellobiose with simple alkyl chains is reported. While thiolactoside hydrogels are robust, thiocellobioside gels are metastable, precipitating over time into fibrous crystals that can be entangled to create pseudo-hydrogels. Rheology confirms the viscoelastic solid nature of these hydrogels with storage moduli ranging from 10–600 kPa. Additionally, thiolactoside hydrogels are thixotropic which is a desirable property for many potential applications. Freeze-fracture electron microscopy of xerogels shows layers of stacked sheets that are entangled into networks. These structures are unique compared to the fibers or ribbons typically reported for hydrogels. Differential scanning calorimetry provides gel-to-liquid phase transition temperatures ranging from 30 to 80 °C. Prodan fluorescence spectroscopy allows assignment of phase transitions in the gels and other lyotropic phases of high concentration samples. Phase diagrams are estimated for all hydrogels at 1–10 wt% from 5 to ≥ 80 °C. These hydrogels represent a series of interesting materials with unique properties that make them attractive for numerous potential applications. 

In this work we investigate the effects of two distinct actuation methods on the hydrodynamics of elastic rectangular plates oscillating at resonance. Plates are driven by plunging motion at the root or actuated by a distributed internal bending moment at Reynolds numbers between 500 and 4000. The latter actuation method represents internally actuated smart materials and emulates the natural ability of swimming animals to continuously change their shapes with muscles. We conduct experiments with plunging elastic plates and piezoelectric plate actuators that are simulated using a fully coupled three-dimensional computational model based on the lattice Boltzmann method. After experimental validation the computational model is employed to probe plate hydrodynamics for a wide range of parameters, including large oscillation amplitudes which prompts nonlinear effects. The comparison between the two actuation methods reveals that, for the same level of tip deflection, externally actuated plates significantly outperform internally actuated plates in terms of thrust production and hydrodynamic efficiency. The reduced performance of internally actuated plates is associated with their suboptimal bending shapes which leads to a trailing edge geometry with enhanced vorticity generation and viscous dissipation. Furthermore, the difference in actuation methods impacts the inertia coefficient characterizing the plate oscillations, especially for large amplitudes. It is found that the inertia coefficient strongly depends on the tip deflection amplitude and the Reynolds number, and actuation method, especially for larger amplitudes. 

Fiber-based flexible piezoelectric composites with interdigitated electrodes, namely Macro-Fiber Composite (MFC) structures, strike a balance between the deformation and actuation force capabilities for effective underwater bio-inspired locomotion. These materials are also suitable for vibration-based energy harvesting toward enabling self-powered electronic components. In this work, we design, fabricate, and experimentally characterize an MFC-based bio-inspired swimmer-energy harvester platform. Following in vacuo and in air frequency response experiments, the proposed piezoelectric robotic fish platform is tested and characterized under water for its swimming performance both in free locomotion (in a large water tank) and also in a closed-loop water channel under imposed flow. In addition to swimming speed characterization under resonant actuation, hydrodynamic thrust resultant in both quiescent water and under imposed flow are quantified experimentally. We show that the proposed design easily produces thrust levels on the order of biological fish with similar dimensions. Overall it produces thrust levels higher than other smart material-based designs (such as soft material-based concepts), while offering geometric scalability and silent operation unlike large scale robotic fish platforms that use conventional and bulky actuators. The performance of this untethered swimmer platform in piezoelectric energy harvesting is also quantified by underwater base excitation experiments in a quiescent water and via vortex induced-vibration (VIV) experiments under imposed flow in a water channel. Following basic resistor sweep experiments in underwater base excitation experiments, VIV tests are conducted for cylindrical bluff body configurations of different diameters and distances from the leading edge of the energy harvesting tail portion. The resulting concept and design can find use for underwater swimmer and sensor applications such as ecological monitoring, among others. 

The rapid progress of proton exchange membrane fuel cells (PEMFCs) and alkaline exchange membrane fuel cells (AMFCs) has boosted the hydrogen economy concept via diverse energy applications in the past decades. For a holistic understanding of the development status of PEMFCs and AMFCs, recent advancements in electrocatalyst design and catalyst layer optimization, along with cell performance in terms of activity and durability in PEMFCs and AMFCs, are summarized here. The activity, stability, and fuel cell performance of different types of electrocatalysts for both oxygen reduction reaction and hydrogen oxidation reaction are discussed and compared. Research directions on the further development of active, stable, and low‐cost electrocatalysts to meet the ultimate commercialization of PEMFCs and AMFCs are also discussed.